Organic-inorganic hybrid lead iodide perovskites are universally recognized as very promising photovoltaic (PV) materials. While outstanding PV performance is continuously reported, manipulating these hybrid perovskites for extraordinary optoelectronic properties with a greater intrinsic structural stability becomes a growing attention. The soft nature of organic-inorganic halide perovskites renders their lattice particularly tunable to external stimuli such as pressure, offering an effective way to modify their structure for extraordinary optoelectronic properties. However, these soft materials meanwhile feature a general characteristic that even a very mild pressure will lead to detrimental lattice distortion and weaken the critical light-matter interaction, thereby triggering the performance degradation.